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• W2279622006 abstract "The electronic metal–substrate interaction plays an important role in the surface reactions on supported metal nanoparticles. We study the interaction between rhodium clusters and cerium oxide substrate having various stoichiometries, CeOx (2.00 > x > 1.67), by means of photoelectron spectroscopy. Our results show that rhodium deposited on substrates with stoichiometry of 2.00 > x > 1.93 induces reduction of cerium oxide. On the other hand, cerium oxide with a higher degree of reduction (1.93 > x > 1.67) becomes partially oxidized after the Rh deposition. Density functional theory simulations of Rh adatom adsorbed on the CeO2(111) surface and on an oxygen vacancy at the CeOx(111) surface show that there is a charge transfer between rhodium and cerium oxide substrate. While Rh adsorption on the CeO2(111) surface leads to electron depletion at the Rh adatom and cerium oxide reduction, Rh adsorption on the oxygen vacancy at CeOx(111) leads to electron accumulation about the Rh adatom and partial oxidation of..." @default.
• W2279622006 created "2016-06-24" @default.
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• W2279622006 date "2016-03-02" @default.
• W2279622006 modified "2023-10-03" @default.
• W2279622006 title "Experimental and Theoretical Study on the Electronic Interaction between Rh Adatoms and CeO_<i>x</i> Substrate in Dependence on a Degree of Cerium Oxide Reduction" @default.
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• W2279622006 doi "https://doi.org/10.1021/acs.jpcc.5b11431" @default.
• W2279622006 hasPublicationYear "2016" @default.
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