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• W2280431368 endingPage "2939" @default.
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• W2280431368 abstract "Significance The excitation energy transfer in light-harvesting complexes is usually studied either by ultrafast bulk spectroscopy or by single-molecule spectroscopy. These methods are to a high degree complementary: Bulk spectroscopy measures ultrafast processes averaged over thousands of complexes, whereas single-molecule spectroscopy observes much slower dynamics in individual complexes. In this work, we combine these approaches using a recently developed ultrafast single-molecule spectroscopy technique. This enables us, for the first time (to our knowledge), to observe ultrafast energy relaxation with a rate around 100 fs in individual light-harvesting complexes. We determine the distribution of the relaxation times, observe changes of the relaxation time in one complex, and find how the relaxation depends on excitation wavelength." @default.
• W2280431368 created "2016-06-24" @default.
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• W2280431368 date "2016-02-22" @default.
• W2280431368 modified "2023-10-12" @default.
• W2280431368 title "Ultrafast energy relaxation in single light-harvesting complexes" @default.
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• W2280431368 doi "https://doi.org/10.1073/pnas.1522265113" @default.
• W2280431368 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4801264" @default.
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• W2280431368 hasPublicationYear "2016" @default.
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