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- W2280732239 abstract "Dissociation recombination in electron-diatomic molecular ion collisions has been described theoretically by a first-order treatment and by two ab-initio fully quantal treatments based on configuration mixing and on multichannel quantum defect theory, respectively. Agreement with experiment is limited to only (e{sup {minus}} - H{sub 2}{sup +}) collisions and possibly to (e{sup {minus}} - N{sub 2}{sup +}) collisions. In an effort (a) to gain further insight into the physics not included in the first-order treatment, and difficult to extract from the numerical quantal procedure; and (b) to see if simple analytical expressions for the recombination rate which are more accurate than the first-order expression can be derived without recourse to the full quantal treatment, a two-state semiclassical theory is presented here. Not only will it be invaluable for the simpler diatomic species, but the present theory can also be applied to cases where curves do not cross and to complex molecular systems." @default.
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- W2280732239 date "1993-12-01" @default.
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- W2280732239 title "Electron-ion dissociative recombination" @default.
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