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- W2280932783 abstract "Aprotic acetamidine {Me2NC(Me)N(R)(CuBr)}2 {R = iPr (2a), Cy (2b), Ph (2c)} and neutral 1,3-P,N phosphaamidine copper bromide complexes {(CuBr)(Ph2PC(Ph)NPh)}4 (6a), {(CuBr)4(Ph2PC(Ph)NiPr)2}·{2CH2Cl2} (6b), (CuBr)4(iPr2PC(Ph)NPh)2} (7a) and {(CuBr)4(iPr2PC(Ph)NiPr)2} (7b) are prepared by direct combination of corresponding amidine and phosphaamidine with CuBr(DMS). X-ray crystallographic analysis of the acetamidine complexes reveal monodentate Nimine coordination to copper with significant degree of delocalization about the NCN framework and a relatively short Cu–Cu interaction of 2.5758(8) Å in 2c compared to (2.9801)(10) Å 2a. The phosphaamidine ligands are never η1–Nimine bound; instead they are η1–P bound in the cubane complex 6a or η2-bound in the step cluster complexes 6b, 7a and 7b." @default.
- W2280932783 created "2016-06-24" @default.
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- W2280932783 date "2016-04-01" @default.
- W2280932783 modified "2023-10-01" @default.
- W2280932783 title "Contrasting connectivity of amidine and phosphaamidine (1,3-P,N) Cu(I) complexes" @default.
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- W2280932783 doi "https://doi.org/10.1016/j.ica.2016.02.024" @default.
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