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• W2282072364 abstract "The electrochemical conversion of carbon dioxide (CO2) into valuable compounds is a promising route toward the valorization of this molecule of high environmental impact. Yet, an industrial process involving CO2 electroreduction is still far from reality and requires deep and fundamental studies for a further understanding and better development of the process. In this work, we describe in situ spectroelectrochemical studies based on Fourier transform infrared spectroscopy and surface-enhanced Raman spectroscopy of the CO2 reduction in acetonitrile solutions at copper electrodes. The influence of factors such as the water content and the supporting electrolyte on the reaction products were evaluated and compared to products obtained on metal electrodes other than Cu, such as Pt, Pb, Au, Pd, and Ag. The results show that at Cu electrodes in acetonitrile containing small amounts of water, the main reaction products from CO2 reduction are carbonate, bicarbonate, and CO. The formation of CO was observed at le..." @default.
• W2282072364 created "2016-06-24" @default.
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• W2282072364 date "2016-03-08" @default.
• W2282072364 modified "2023-10-03" @default.
• W2282072364 title "In Situ Spectroscopic Study of CO₂ Electroreduction at Copper Electrodes in Acetonitrile" @default.
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• W2282072364 doi "https://doi.org/10.1021/acscatal.5b02543" @default.
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