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- W2283009411 abstract "Abstract Structure–activity relationships of amorphous (a-), tetragonal (t-), monoclinic (m-) ZrO 2 phase supported copper catalysts for methanol synthesis from CO 2 hydrogenation were investigated with X-ray diffraction (XRD), high resolution transmission electron microscopy (HR-TEM), N 2 O chemisorption, H 2 -temperature programmed reduction (H 2 -TPR), X-ray absorption spectroscopy (XAS), H 2 and CO 2 temperature-programmed desorption (H 2 - and CO 2 -TPD). The order of copper surface area is found to be as follows: Cu/a-ZrO 2 > Cu/t-ZrO 2 > Cu/m-ZrO 2 . The increased yield of methanol is correlated to the increase of copper surface area. However, normalization of the copper site specific activity (TOF methanol ) of Cu/t-ZrO 2 is about 1.10–1.50 times and 1.62–3.59 times higher than Cu/a-ZrO 2 and Cu/m-ZrO 2 , respectively. The high TOF methanol is caused by a strong Cu–ZrO 2 interaction and a high surface concentration of atomic hydrogen to CO 2 ." @default.
- W2283009411 created "2016-06-24" @default.
- W2283009411 creator A5003532951 @default.
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- W2283009411 creator A5008872657 @default.
- W2283009411 creator A5011184320 @default.
- W2283009411 creator A5050660623 @default.
- W2283009411 date "2016-06-01" @default.
- W2283009411 modified "2023-10-17" @default.
- W2283009411 title "CO 2 hydrogenation to methanol over Cu/ZrO 2 catalysts: Effects of zirconia phases" @default.
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- W2283009411 doi "https://doi.org/10.1016/j.cej.2016.02.069" @default.
- W2283009411 hasPublicationYear "2016" @default.
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