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• W2283177130 abstract "The prototypical single-molecule magnet (SMM) molecule [Mn12O12(O2CCH3)16(OH2)4] was incorporated under mild conditions into a highly porous metal–organic framework (MOF) matrix as a proof of principle for controlled nanostructuring of SMMs. Four independent experiments revealed that the SMM clusters were successfully loaded in the MOF pores, namely synchrotron-based powder diffraction, physisorption analysis, and in-depth magnetic and thermal analyses. The results provide incontrovertible evidence that the magnetic composite, SMM@MOF, combines key SMM properties with the functional properties of MOFs. Most importantly, the incorporated SMMs exhibit a significantly enhanced thermal stability with SMM loading advantageously occurring at the periphery of the bulk MOF crystals with only a single SMM molecule isolated in the transverse direction of the pores." @default.
• W2283177130 created "2016-06-24" @default.
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• W2283177130 date "2015-07-15" @default.
• W2283177130 modified "2023-10-18" @default.
• W2283177130 title "Metal–Organic Frameworks as Platforms for the Controlled Nanostructuring of Single-Molecule Magnets" @default.
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• W2283177130 doi "https://doi.org/10.1021/jacs.5b06002" @default.
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• W2283177130 hasPublicationYear "2015" @default.
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