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• W2284291658 abstract "Experimental data from the decomposition of hydrogen peroxide by the Fe(III) initiated Fenton reaction at pH 3 were compared with model predictions. This model used only defined chemical reactions, their published rate constants, the initial reactant concentrations, and no fitting parameters. The initial concentration of hydrogen peroxide ranged from 0.1-1 millimolar, and the amount of Fe(III) used varied from 4-325 micromolar. Differences between the data and model results ranged from insignificant to about 20 percent of the initial concentration of hydrogen peroxide. In the second set of experiments, 14C-labeled formic acid, a hydroxyl radical probe, was added. Model results of hydrogen peroxide and 14C loss over time again compared favorably with experimental data. The steady state concentration of hydroxyl radicals calculated from the 14C-labeled formic acid agreed with those predicted by the model to within a factor of two or better. These values were also compared with those derived from steady state approximations. Furthermore, it was shown that the degradation rate of the 14C-labeled formic acid could be predicted from the decomposition rate of hydrogen peroxide. Thesis Supervisor: Bettina M. Voelker Title: Assistant Professor of Civil and Environmental Engineering" @default.
• W2284291658 created "2016-06-24" @default.
• W2284291658 creator A5040959366 @default.
• W2284291658 date "1999-01-01" @default.
• W2284291658 modified "2023-09-28" @default.
• W2284291658 title "KINETICS OF THE Fe(III) INITIATED DECOMPOSITION OF HYDROGEN PEROXIDE: EXPERIMENTAL AND MODEL RESULTS" @default.
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