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• W2284393609 abstract "Many promising nanophotonics endeavours hinge upon the unique plasmonic properties of nanometallic structures with narrow non-metallic gaps, which support super-concentrated bonding modes that singularly redshift with decreasing separations. In this letter, we present a descriptive physical picture, complemented by elementary asymptotic formulae, of a nonlocal mechanism for plasmon-redshift saturation at subnanometric gap widths. Thus, by considering the electron-charge and field distributions in the close vicinity of the metal-vacuum interface, we show that nonlocality is asymptotically manifested as an effective potential discontinuity. For bonding modes in the near-contact limit, the latter discontinuity is shown to be effectively equivalent to a widening of the gap. As a consequence, the resonance-frequency near-contact asymptotics are a renormalisation of the corresponding local ones. Specifically, the renormalisation furnishes an asymptotic plasmon-frequency lower bound that scales with the $1/4$-power of the Fermi wavelength. We demonstrate these remarkable features in the prototypical cases of nanowire and nanosphere dimers, showing agreement between our elementary expressions and previously reported numerical computations." @default.
• W2284393609 created "2016-06-24" @default.
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• W2284393609 date "2016-01-13" @default.
• W2284393609 modified "2023-09-30" @default.
• W2284393609 title "Asymptotics of surface-plasmon redshift saturation at subnanometric separations" @default.
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• W2284393609 doi "https://doi.org/10.1103/physrevb.93.041409" @default.
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