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- W2285151572 abstract "We present a method to measure rotational transitions of molecular anions in the terahertz domain by sequential two-photon absorption. Ion excitation by bound-bound terahertz absorption is probed by absorption in the visible on a bound-free transition. The visible frequency is tuned to a state-selective photodetachment transition of the excited anions. This provides a terahertz action spectrum for just few hundred molecular ions. To demonstrate this we measure the two lowest rotational transitions, J=1<-0 and J =2<-1 of OD- anions in a cryogenic 22-pole trap. We obtain rotational transition frequencies of 598596.08(19) MHz for J=1<-0 and 1196791.57(27) MHz for J=2<-1 of OD-, in good agreement with their only previous measurement. This two-photon scheme opens up terahertz rovibrational spectroscopy for a range of molecular anions, in particular for polyatomic and cluster anions." @default.
- W2285151572 created "2016-06-24" @default.
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- W2285151572 date "2016-03-21" @default.
- W2285151572 modified "2023-09-25" @default.
- W2285151572 title "Terahertz-visible two-photon rotational spectroscopy of cold<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow><mml:mi>OD</mml:mi></mml:mrow><mml:mo>−</mml:mo></mml:msup></mml:math>" @default.
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- W2285151572 doi "https://doi.org/10.1103/physreva.93.032513" @default.
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