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- W2286615387 abstract "The adsorption of a close-packed ${mathrm{C}}_{60}$ single layer on the clean $c(2ifmmodetimeselsetexttimesfi{}8)ensuremath{-}mathrm{Ge}(111)$ surface leads to the formation of a $3sqrt{3}ifmmodetimeselsetexttimesfi{}3sqrt{3}R30ifmmode^circelsetextdegreefi{}$ low-energy electron diffraction pattern upon annealing at 450--500 ifmmode^circelsetextdegreefi{}C. We have investigated this phase using synchrotron-radiation photoemission. The $mathrm{Ge}3d$ core-level spectra show the quenching of the surface features related to the adatoms/rest-atoms complex of the original $mathrm{Ge}(111)ensuremath{-}c(2ifmmodetimeselsetexttimesfi{}8)$ reconstruction, suggesting that the observed $3sqrt{3}ifmmodetimeselsetexttimesfi{}3sqrt{3}R30ifmmode^circelsetextdegreefi{}$ ordering is not due to a Ge(111) reconstruction induced by the ${mathrm{C}}_{60}$ adsorption, as instead previously argued on the basis of scanning tunneling microscopy measurements. Moreover, no filling of the lowest unoccupied molecular orbital derived bands has been observed. The C $1s$ core level and the valence-band photoemission spectra point to the presence of a localized covalent bond between the ${mathrm{C}}_{60}$ molecules and the Ge atoms. This bond induces the splitting of the ${mathrm{C}}_{60}$ highest occupied molecular orbital with a feature appearing at about 2.3 eV." @default.
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- W2286615387 date "2000-04-15" @default.
- W2286615387 modified "2023-10-03" @default.
- W2286615387 title "Interaction ofC60with Ge(111) in the33×33R30°phase: A(2×2)model" @default.
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- W2286615387 doi "https://doi.org/10.1103/physrevb.61.10411" @default.
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