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• W2287581953 abstract "Large-scale production of hydrogen gas by water electrolysis is hindered by the sluggish kinetics of oxygen evolution reaction (OER) at the anode. The development of a highly active and stable catalyst for OER is a challenging task. Electrochemically prepared amorphous metal-based catalysts have gained wide attention after the recent discovery of a cobalt-phosphate (Co-Pi) catalyst. Herein, an amorphous iridium-phosphate (Ir-Pi) is investigated as an oxygen evolution catalyst. The catalyst is prepared by the anodic polarization of carbon paper electrodes in neutral phosphate buffer solutions containing IrCl3. The Ir-Pi film deposited on the substrate has significant amounts of phosphate and Ir centers in an oxidation state higher than +4. Phosphate plays a significant role in the deposition of the catalyst and also in its activity toward OER. The onset potential of OER on the Ir-Pi is about 150 mV lower in comparison with the Co-Pi under identical experimental conditions. Thus, Ir-Pi is a promising catalyst for electrochemical oxidation of water." @default.
• W2287581953 created "2016-06-24" @default.
• W2287581953 creator A5057455650 @default.
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• W2287581953 date "2015-07-14" @default.
• W2287581953 modified "2023-10-16" @default.
• W2287581953 title "High Catalytic Activity of Amorphous Ir-Pi for Oxygen Evolution Reaction" @default.
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• W2287581953 doi "https://doi.org/10.1021/acsami.5b02601" @default.
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