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- W2287642238 abstract "The asymmetric synthesis of functionalized nitrocyclopropanes has been achieved by a one-pot, four-step method catalyzed by (S)-diphenylprolinol TMS ether, which joins two sequential domino reactions, namely a domino sulfa-Michael/aldol condensation of α,β-unsaturated aldehydes with 1,4-dithiane-2,5-diol, and a domino Michael/α-alkylation reaction of the derived chiral dihydrothiophenes with bromonitromethane. The title compounds were obtained in 27–45% yields, with high levels of diastereoselectivity (93:7 to 100:0 dr) and generally good enantioselectivities (up to 95:5 er)." @default.
- W2287642238 created "2016-06-24" @default.
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- W2287642238 date "2015-09-09" @default.
- W2287642238 modified "2023-10-18" @default.
- W2287642238 title "One-Pot, Four-Step Organocatalytic Asymmetric Synthesis of Functionalized Nitrocyclopropanes" @default.
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- W2287642238 doi "https://doi.org/10.1021/acs.joc.5b01607" @default.
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