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- W2289075291 abstract "A new approach to functionalized γ-butenolides based on reagent-controlled tandem reaction sequences of Morita–Baylis–Hillman-type vinyl epoxides is described. The nucleophilic addition of a tertiary phosphine to the electron-deficient alkene led to ring-opening of the epoxide followed by lactonization to produce phosphonium ylides, which could undergo Wittig olefination with aryl trifluoromethyl ketones and aryl aldehydes to give 3-alkenyl γ-butenolides in moderate to good yields and high E/Z selectivity. Tertiary amine promoted the Michael-type addition of carbon- and nitrogen-based nucleophiles to the vinyl epoxides followed by lactonization to provide diverse 3-substituted γ-butenolides." @default.
- W2289075291 created "2016-06-24" @default.
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- W2289075291 date "2016-03-04" @default.
- W2289075291 modified "2023-10-09" @default.
- W2289075291 title "Reagent-Controlled Tandem Reactions of Vinyl Epoxides: Access to Functionalized γ-Butenolides" @default.
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- W2289075291 doi "https://doi.org/10.1021/acs.orglett.6b00392" @default.
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