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• W2290076645 abstract "Photocatalysts based on g-C3N4 by loading cocatalysts or constructing heterojunctions have shown great potential in solar-driven water oxidation. However, the intrinsic drawbacks of g-C3N4, such as poor mass diffusion and charge separation efficiency, remain as the bottleneck to achieve highly efficient water oxidation. Here we report a simple protonation method to improve the activity of g-C3N4. Studies using valence band X-ray photoelectron spectra and steady-state and time-resolved spectroscopy reveal that the promotion of catalytic ability originates from the higher thermodynamical driving force and longer-lived charge separation state, which may provide guidance in designing efficient polymeric semiconductor photocatalysts with desirable kinetics for water oxidation." @default.
• W2290076645 created "2016-06-24" @default.
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• W2290076645 date "2015-10-23" @default.
• W2290076645 modified "2023-10-16" @default.
• W2290076645 title "Enhanced Driving Force and Charge Separation Efficiency of Protonated g-C₃N₄ for Photocatalytic O₂ Evolution" @default.
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• W2290076645 doi "https://doi.org/10.1021/acscatal.5b02185" @default.
• W2290076645 hasPublicationYear "2015" @default.
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