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- W2291587229 abstract "Hydrogen-bonding organocatalysis has emerged as a promising biomimetic alternative to Lewis acid catalysis. Urea, thiourea and squaramide moieties represent the most common hydrogen-bond donors used for the preparation of these catalysts. However, their significant tendency to undergo self-quenching (self-aggregation) often decreases their solubility and reactivity. Recently, scientists have found a promising way around this problem by immobilizing the hydrogen-bonding organocatalysts on metal–organic frameworks (MOFs). Along with advantageous modular synthesis and recycling properties, the tunable porosity and topology of MOFs also allows fast mass transport and/or interactions with substrates. Herein, we highlight the existing examples dealing with the fabrication and testing of hydrogen-bonding organocatalyst-containing MOFs, providing also our vision for further advances in this area. The results derived from these studies will likely serve as inspiration for the future development of superior hydrogen-bonding organocatalysts to accomplish in confined spaces chemical transformations that are either slow or unaffordable under standard homogeneous conditions." @default.
- W2291587229 created "2016-06-24" @default.
- W2291587229 creator A5026887247 @default.
- W2291587229 creator A5052028748 @default.
- W2291587229 creator A5083037509 @default.
- W2291587229 creator A5085603418 @default.
- W2291587229 date "2016-01-01" @default.
- W2291587229 modified "2023-10-16" @default.
- W2291587229 title "Metal–organic frameworks (MOFs) bring new life to hydrogen-bonding organocatalysts in confined spaces" @default.
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- W2291587229 doi "https://doi.org/10.1039/c5ce02526e" @default.
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