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- W2292012253 abstract "High calcination temperatures are often required in nanoparticle synthesis and an understanding of how heating affects the structure and chemical arrangement of bimetallic nanoclusters is essential to design efficient fabrication processes. We have investigated the kinetic stability of 147-atom Au–Ag nanoalloys with varying composition and chemical ordering using ensemble molecular dynamics simulations to replicate these high temperature conditions. Ag-rich mixed alloys undergo a diffusion-less “martensitic” structural transition from cuboctahedral to icosahedral; the melting temperature (Tm) of the subsequent icosahedra is dependent on the Au:Ag stoichiometry. Core@shell chemical arrangements do not behave in a similar manner: Tm strongly depends on the shell component; additionally Au55@Ag92 exhibits increased stability as a result of its icosahedral Au core. We also report a novel dependence of nanocluster phase transitions on the chemical arrangement, as shown by low temperature nonmartensitic atomic ..." @default.
- W2292012253 created "2016-06-24" @default.
- W2292012253 creator A5002437738 @default.
- W2292012253 creator A5042572313 @default.
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- W2292012253 date "2015-10-02" @default.
- W2292012253 modified "2023-10-12" @default.
- W2292012253 title "Influence of Composition and Chemical Arrangement on the Kinetic Stability of 147-Atom Au–Ag Bimetallic Nanoclusters" @default.
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- W2292012253 doi "https://doi.org/10.1021/acs.jpcc.5b03577" @default.
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