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• W2292518915 abstract "Abstract Production of chemical fuels by solar‐driven thermochemical cycling has recently generated significant interest for its potential as a highly efficient method of storing solar energy. Of particular interest is the thermochemical process using non‐stoichiometric oxides, such as ceria. In this process a reactive oxide is cyclically exposed to an inert gas, typically at 1500 °C to induce the partial reduction of the oxide, and then exposed to an oxidizing gas of either H 2 O or CO 2 at a temperature between 800–1500 °C to oxidize the oxide and release H 2 or CO. Conventional wisdom has held that material kinetics limit the fuel production rates. Herein we demonstrate that, instead, at 1500 °C the rates of both reduction and oxidation of ceria, and hence also the global fuel production rate, are limited only by thermodynamic considerations for any reasonable set of operating conditions. Thus, in terms of materials design, significant room exists for sacrificing material kinetics in favor of thermodynamic characteristics." @default.
• W2292518915 created "2016-06-24" @default.
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• W2292518915 date "2016-02-23" @default.
• W2292518915 modified "2023-10-18" @default.
• W2292518915 title "Implications of Exceptional Material Kinetics on Thermochemical Fuel Production Rates" @default.
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• W2292518915 doi "https://doi.org/10.1002/ente.201500506" @default.
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