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• W2293376293 abstract "Abstract A new multicomponent coupling reaction for the enantioselective synthesis of pyrrolo[1,2‐ a ]indoles under the catalysis of a chiral disulfonimide is described. The high specificity of the reaction is a consequence of the multidentate character of the Brønsted acid catalyst. Insights from DFT calculations helped explain the unexpected high enantioselectivity observed with the simplest 3,3′‐unsubstituted binaphthyl catalyst as a result of transition‐state stabilization by a network of cooperative noncovalent interactions. The remarkable enantioinversion resulting from the simple introduction of substituents at 3‐ and 3′‐positions, the first reported example of this phenomenon in the context of binaphthalene‐derived Brønsted acid catalysis, was instead attributed to destabilizing steric interactions." @default.
• W2293376293 created "2016-06-24" @default.
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• W2293376293 date "2016-02-02" @default.
• W2293376293 modified "2023-10-14" @default.
• W2293376293 title "Exploiting the Multidentate Nature of Chiral Disulfonimides in a Multicomponent Reaction for the Asymmetric Synthesis of Pyrrolo[1,2‐<i>a</i>]indoles: A Remarkable Case of Enantioinversion" @default.
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• W2293376293 doi "https://doi.org/10.1002/anie.201511231" @default.
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• W2293376293 hasPublicationYear "2016" @default.
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