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• W2293655362 startingPage "2770" @default.
• W2293655362 abstract "A formal palladium-catalyzed aerobic bimolecular carbocyclization reaction of (Z)-hexa-1,5-diyn-3-ene scaffolds has been successfully developed for the construction of 2,6-diacylnaphthalenes, wherein copper salts play a critical role in accomplishing the oxygenative homo- and hetero-dimerization processes of readily accessible enediyne–carboxylic acids and esters, respectively. The enediyne dimerization protocol provides a flexible and regiospecific approach to a variety of functionalized naphthalenes with up to six differentiated substituents in good yields by using a directing-group-assisted coupling and decoupling strategy. Mechanistic studies indicated that the two oxygen atoms being selectively incorporated into the crossover-annulation products of enediynecarboxylic acid and ester directly originate from atmospheric molecular oxygen and H2O, respectively." @default.
• W2293655362 created "2016-06-24" @default.
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• W2293655362 date "2016-03-15" @default.
• W2293655362 modified "2023-10-17" @default.
• W2293655362 title "Coupling and Decoupling Approach Enables Palladium-Catalyzed Aerobic Bimolecular Carbocyclizations of Enediynes to 2,6-Diacylnaphthalenes" @default.
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• W2293655362 doi "https://doi.org/10.1021/acs.joc.5b02870" @default.
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• W2293655362 hasPublicationYear "2016" @default.
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