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• W2296447809 abstract "The high strain-rate rheological and mechanical properties of bi-modal epoxy polymer networks were characterized using molecular dynamics simulation. The complex Young's modulus was found by applying a cyclic sinusoidal strain over a wide range of temperatures spanning the glass transition. The non-linear stress response was studied in the glass transition region using uni-axial deformation. We discuss special considerations in computing viscoelastic properties at the high strain-rates available to molecular dynamics. As in experimental studies, the complex modulus is shown to be a function of the network composition and strain rate. However, the high strain-rate simulations performed here predict the existence of broad peaks in the temperature-dependent loss modulus and slow relaxation of the storage modulus. In general, it is observed that network compositions with larger amounts of short, stiff 4,4’-methylenebis(cyclohexylamine) (MCA) cross-linkers lead to an increase in the mechanical glass transition temperature as well as the breadth of the glass transition compared to longer, more flexible poly(oxypropylene) diamine (POP) cross-linkers. When the networks of any composition were deformed beyond the linear region, the stress response displayed a plateau that was associated with the extension of network chains." @default.
• W2296447809 created "2016-06-24" @default.
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• W2296447809 date "2016-05-01" @default.
• W2296447809 modified "2023-10-01" @default.
• W2296447809 title "Bi-modal polymer networks: Viscoelasticity and mechanics from molecular dynamics simulation" @default.
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• W2296447809 doi "https://doi.org/10.1016/j.polymer.2016.03.024" @default.
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