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- W2296759712 abstract "2/ scattering was studied in the relative energy range of 0.74 to 30. eV. The Na/sup +/ -- D/sub 2/ system shows predominantly vibrationally elastic scattering below 8 eV relative energy. Above 8 eV the most probable inelasticity observed increases monotonically with the initial collision energy and is comparable to excitation to higher vibrational levels. At 17 eV this inelasticity is 3.92 eV. Classical trajectory calculations are used to study the contribution of different collision orientations to the scattering spectra. It is found that collisions in which the projectile approaches the molecule along the bisector of its bond yield the most significant contribution to the backscattering spectra. It is shown that all backscattering can be accounted for by considering only zero impact parameter collisions. The results of trajectory calculations using a dumbbell repulsive ion molecule interaction potential on collisions restricted to zero impact parameter are fit to the experimental data. Through the discrepancies in the fit it is found that the ratio of the stiffness of the interaction potential along the collinear axis to that in the molecular bisector plane is greater than that ratio for the dumbbell potential. (auth)" @default.
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- W2296759712 date "1971-04-01" @default.
- W2296759712 modified "2023-10-14" @default.
- W2296759712 title "Dynamic isotope effects in ion-molecule reactions" @default.
- W2296759712 doi "https://doi.org/10.2172/4029871" @default.
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