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- W2298653941 abstract "The standard closed-orbit theory is extended for the photodetachment of negative ions in a time-dependent electric field. The time-dependent photodetachment rate is specifically studied in the presence of a single-cycle terahertz pulse, based on exact quantum simulations and semiclassical analysis. We find that the photodetachment rate is unaffected by a weak terahertz field, but oscillates complicatedly when the terahertz pulse gets strong enough. Three types of closed classical orbits are identified for the photoelectron motion in a strong single-cycle terahertz pulse, and their connections with the oscillatory photodetachment rate are established quantitatively by generalizing the standard closed-orbit theory to a time-dependent form. By comparing the negative hydrogen and fluorine ions, both the in-phase and antiphase oscillations can be observed, depending on a simple geometry of the contributed closed classical orbits. On account of its generality, the presented theory provides an intuitive understanding from a time-dependent viewpoint for the photodetachment dynamics driven by an external electric field oscillating at low frequency." @default.
- W2298653941 created "2016-06-24" @default.
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- W2298653941 date "2016-05-17" @default.
- W2298653941 modified "2023-10-01" @default.
- W2298653941 title "Closed-orbit theory for photodetachment in a time-dependent electric field" @default.
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- W2298653941 doi "https://doi.org/10.1103/physreva.93.053413" @default.
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