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• W2298664441 abstract "The synthesis and structural determination of the first thorium phosphinidene complex are reported. The reaction of 2 equiv of (C5Me5)2Th(CH3)2 with H2P(2,4,6-iPr3C6H2) at 95 °C produces [(C5Me5)2Th]2(μ2-P[(2,6-CH2CHCH3)2-4-iPrC6H2] as well as 4 equiv of methane, 2 equiv from deprotonation of the phosphine and 2 equiv from C–H bond activation of one methyl group of each of the isopropyl groups at the 2- and 6-positions. Transition state calculations indicate that the steps in the mechanism are P–H, C–H, C–H, and then P–H bond activation to form the phosphinidene." @default.
• W2298664441 created "2016-06-24" @default.
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• W2298664441 date "2015-11-17" @default.
• W2298664441 modified "2023-10-03" @default.
• W2298664441 title "Formation of a Bridging Phosphinidene Thorium Complex" @default.
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• W2298664441 doi "https://doi.org/10.1021/jacs.5b09826" @default.
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