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- W2300620488 abstract "Precisely tailoring surface chemistry of layered materials is a growing need for fields ranging from electronics to biology. For many applications, the need for noncovalently adsorbed ligands to simultaneously control interactions with a nonpolar substrate and a polar solvent is a particular challenge. However, biology routinely addresses a similar challenge in the context of the lipid bilayer. While conventional standing phases of phospholipids (such as those found in a bilayer) would not provide spatially ordered interactions with the substrate, here we demonstrate formation of a sitting phase of polymerizable phospholipids, in which the two alkyl chains extend along the surface and the two ionizable functionalities (a phosphate and an amine) sit adjacent to the substrate and project into the solvent, respectively. Interfacial ordering and polymerization are assessed by high-resolution scanning probe measurements. Water contact angle titrations demonstrate interfacial pKa shifts for the lipid phosphate but not for the amine, supporting localization of the phosphate near the nonpolar graphite surface." @default.
- W2300620488 created "2016-06-24" @default.
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- W2300620488 date "2016-03-24" @default.
- W2300620488 modified "2023-09-24" @default.
- W2300620488 title "Sitting Phases of Polymerizable Amphiphiles for Controlled Functionalization of Layered Materials" @default.
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- W2300620488 doi "https://doi.org/10.1021/jacs.5b13179" @default.
- W2300620488 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26974686" @default.
- W2300620488 hasPublicationYear "2016" @default.
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