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- W2300943203 abstract "In a mixed solvent of water and dimethylformamide (DMF), porphyrin molecules have two types of orientation, tilted and parallel, toward a surface of silicate nanosheet. In the solvent, tilted species have lower energy. The Tn ← T1 absorption of porphyrin molecules adsorbed at the surface of the nanosheet in the mixed solvent was observed at five different temperatures. The decay curve was analyzed with an equation for transient absorption difference, describing the behavior of parallel and tilted adsorbed species in the ground state and excited state to determine the rate constants for the orientation change and the radiationless deactivation. The rate constants of the orientation change increased with the temperature. The activation energy and energy gap between parallel and tilted species were estimated by analyzing the temperature dependence of the rate constants. The energy gap obtained in this kinetic study was consistent with our thermodynamically obtained value previously reported." @default.
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- W2300943203 date "2016-03-23" @default.
- W2300943203 modified "2023-09-25" @default.
- W2300943203 title "Kinetic Analysis by Laser Flash Photolysis of Porphyrin Molecules’ Orientation Change at the Surface of Silicate Nanosheet" @default.
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- W2300943203 doi "https://doi.org/10.1021/acs.jpcc.6b01211" @default.
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