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• W2307830008 abstract "Abstract In this study, Ce-doped zirconolite-rich ceramics were prepared by solid-state reaction process using cerium as the surrogate of tetravalence actinide nuclide. The occupancy of Ce in the waste forms was investigated. The aqueous durability of Ce-doped zirconolite-rich ceramic was examined as well. The results show that zirconolite and pseudobrookite coexisted after being sintered at 1200 °C for 6 h. Meanwhile, perovskite is inevitable generated during the process. CeO 2 can be successfully incorporated into the lattice structure of the zirconolite-rich ceramics. The maximum containing capacity of CeO 2 is up to 14.95 wt% or y  = 0.4. The normalized elemental leaching rates of Ce and Ca are fairly constant in low values of 1.2 × 10 −6 and 2.3 × 10 −2  g m −2  d −1 after 28 days. The normalized leaching rate of Fe is also in a low value of 2.9 × 10 −4  g m −2  d −1 after 7 days." @default.
• W2307830008 created "2016-06-24" @default.
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• W2307830008 date "2015-11-01" @default.
• W2307830008 modified "2023-09-24" @default.
• W2307830008 title "Solid-state reaction synthesis and aqueous durability of Ce-doped zirconolite-rich ceramics" @default.
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• W2307830008 doi "https://doi.org/10.1016/j.jnucmat.2015.07.047" @default.
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