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• W2308197831 abstract "The mechanical and viscoelastic responses of poly(ethyl methacrylate) (PEMA) ultrathin films over thicknesses ranging from 21 to 112 nm have been studied using a nanobubble inflation method. The stress–strain response of the PEMA thin films shows a rubbery stiffening as the film thickness decreases, and the present results are combined with prior measurements of the rubbery stiffening index S for multiple polymers. We find that S is linearly correlated with the dynamic fragility index m. The results are also consistent with expectation from Ngai et al.’s [J. Polym. Sci., Part B: Polym. Phys. 2013, 51 (3)] recent proposition based on his coupling model but do not seem to correlate with the molecular composite concept proposed by Page et al. [Nano Lett. 2014, 14 (5)] as a means to explain the dependence of the rubbery stiffening on chemical structure of the polymer. In addition, we observe a reduction in glass transition temperature of as much as 15.7 K for PEMA films of 21 nm thickness." @default.
• W2308197831 created "2016-06-24" @default.
• W2308197831 creator A5047596738 @default.
• W2308197831 creator A5082965591 @default.
• W2308197831 date "2015-08-18" @default.
• W2308197831 modified "2023-09-30" @default.
• W2308197831 title "Ultrathin Polymer Films: Rubbery Stiffening, Fragility, and <i>T</i>_g Reduction" @default.
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• W2308197831 doi "https://doi.org/10.1021/acs.macromol.5b01263" @default.
• W2308197831 hasPublicationYear "2015" @default.
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