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• W2308351272 abstract "Using Brillouin scattering, we measured the single-crystal elastic constants (Cij’s) of a prototypical metal-organic framework (MOF): zeolitic imidazolate framework (ZIF)-8 [Znð2-methylimidazolateÞ2], which adopts a zeolitic sodalite topology and exhibits large porosity. Its Cij’s under ambient conditions are (in GPa) C11 ¼ 9:522ð7Þ, C12 ¼ 6:865ð14Þ, and C44 ¼ 0:967ð4Þ. Tensorial analysis of the Cij’s reveals the complete picture of the anisotropic elasticity in cubic ZIF-8. We show that ZIF-8 has a remarkably low shear modulus Gmin & 1 GPa, which is the lowest yet reported for a single-crystalline extended solid. Using ab initio calculations, we demonstrate that ZIF-8’s Cij’s can be reliably predicted, and its elastic deformation mechanism is linked to the pliant ZnN4 tetrahedra. Our results shed new light on the role of elastic constants in establishing the structural stability of MOF materials and thus their suitability for practical applications." @default.
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• W2308351272 date "2012-01-01" @default.
• W2308351272 modified "2023-10-12" @default.
• W2308351272 title "ExceptionallyLowShearModulusinaPrototypicalImidazole-BasedMetal-OrganicFramework" @default.
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• W2308351272 hasPublicationYear "2012" @default.
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