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• W2308469968 abstract "Our earlier theoretical calculation and preliminary experiment highlighted LiZnPS4 as a good mid-infrared (mid-IR) nonlinear optical (NLO) material. However, this compound suffers from problems including corrosion of the silica tubes, a pungent smell, deliquescence, and incongruent-melting behavior in the further single crystal growth and applications. In order to overcome these problems, herein, we investigate the analogues of LiZnPS4 and propose that AgZnPS4 would be a good candidate. The combination of experimental and theoretical study demonstrates that AgZnPS4 exhibits a much stronger NLO effect than that of LiZnPS4 despite the relatively smaller energy band gap. More importantly, AgZnPS4 melts congruently with a melting point as low as 534 °C, much lower than those of traditional IR NLO crystals, and is nondeliquescent with enough stability in the air. Such a good crystal growth habit and chemical stability enable AgZnPS4 to possess much better overall performance for the practical mid-IR NLO applications." @default.
• W2308469968 created "2016-06-24" @default.
• W2308469968 creator A5005274481 @default.
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• W2308469968 date "2016-03-25" @default.
• W2308469968 modified "2023-10-16" @default.
• W2308469968 title "Midinfrared Nonlinear Optical Thiophosphates from LiZnPS₄ to AgZnPS₄: A Combined Experimental and Theoretical Study" @default.
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• W2308469968 doi "https://doi.org/10.1021/acs.inorgchem.6b00517" @default.
• W2308469968 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27015097" @default.
• W2308469968 hasPublicationYear "2016" @default.
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