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- W2310588404 abstract "In the process of direct conversion of ethylene to butadiene (flowtype unit, T-973 K, P(C{sub 2}H{sub 2})=10.1 kPa), testing was conducted of aluminosilicate systems having a roughly constant silicate modulus and diverse crystallinity K (K=0, 15, 55, 70, 90). It was found that with increasing K the rate of total C{sub 2}H{sub 4} conversion increased and desired product selectivity essentially decreased from 39.5 to 2.4%. The effect was studied of various factors (temperature, ethylene partial pressure, contact time, reactor free space, the chemical nature of the catalyst surface) on the ethylene conversion pattern both in the presence and absence of catalysts (T=773-1023 K, P(C{sub 2}H{sub 4}) = 1.9-15.4 kPa, F=30-160 ml/min). A heterogeneous-homogeneous mechanism for the reaction progress was suggested and the probable reaction steps were discussed. The optimal reaction conditions have been determined for the direct ethylene-to-butadiene conversion over amorphous aluminosilicate." @default.
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- W2310588404 date "1995-12-31" @default.
- W2310588404 modified "2023-09-23" @default.
- W2310588404 title "Direct ethylene-to-butadiene conversion over aluminosilicates: Effect of catalyst crystallinity" @default.
- W2310588404 hasPublicationYear "1995" @default.
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