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• W2313372478 startingPage "18973" @default.
• W2313372478 abstract "Spin accommodation is demonstrated to play a determining role in the reactivity of silver cluster anions with oxygen. Odd-electron silver clusters are found to be especially reactive, while the anionic 13-atom cluster exhibits unexpected stability against reactivity with oxygen. Theoretical studies show that the odd-even selective behavior is correlated with the excitation needed to activate the O-O bond in O(2). Furthermore, by comparison with the reactivity of proximate even-electron clusters, we demonstrate that the inactivity of Ag(13)(-) is associated with its large spin excitation energy, ascribed to a crystal-field-like splitting of the orbitals caused by the bilayer atomic structure, which induces a large gap despite not having a magic number of valence electrons." @default.
• W2313372478 created "2016-06-24" @default.
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• W2313372478 date "2012-11-07" @default.
• W2313372478 modified "2023-10-18" @default.
• W2313372478 title "Spin Accommodation and Reactivity of Silver Clusters with Oxygen: The Enhanced Stability of Ag₁₃^–" @default.
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• W2313372478 doi "https://doi.org/10.1021/ja303268w" @default.
• W2313372478 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23113750" @default.
• W2313372478 hasPublicationYear "2012" @default.
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