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- W2313449622 abstract "We have obtained the high-resolution threshold photoelectron (TPE) spectra of chlorobenzene C6H5Cl (X1A1), propargyl radical C3H3 (X2B1), and allyl radical C3H5 (X2A1) by employing the vacuum ultraviolet (VUV) laser velocity-map-imaging-TPE (VUV-VMI-TPE) method. The photoelectron energy resolution of 1–2 cm−1 observed for the VUV-VMI-TPE method is comparable to that achieved in VUV laser pulsed-field ionization-photoelectron (VUV-PFI-PE) measurements. Similar to VUV-PFI-PE measurements, the energy resolutions for VUV-VMI-photoelectron (VUV-VMI-PE) and VUV-VMI-TPE measurements are found to depend on the dc electric field F in V/cm used at the photoionization region for electron extraction. The decrease of the ionization thresholds of C6H5Cl and C3H3 observed as a function of F shows that the Stark shift correction for VUV-VMI-TPE measurements is governed by the formula −3.1F in cm−1, which is half of the classical prediction of −6.1F in cm−1. We have also measured the VUV-VMI-PE spectra of C6H5Cl and C3H5 ..." @default.
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- W2313449622 date "2016-02-27" @default.
- W2313449622 modified "2023-10-18" @default.
- W2313449622 title "High-Resolution Threshold Photoelectron Spectroscopy by Vacuum Ultraviolet Laser Velocity-Map-Imaging Method" @default.
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- W2313449622 doi "https://doi.org/10.1063/1674-0068/29/cjcp1512247" @default.
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