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• W2313790876 endingPage "2006" @default.
• W2313790876 startingPage "2000" @default.
• W2313790876 abstract "The reactivity of diaurated species toward nucleophiles was investigated. The reaction yields vinyl gold species and is described as simple SN2 ligand exchange at gold. Using suitably strong nucleophiles, equilibrium constants were determined to measure the stability of various diaurated species. On the basis of these equilibrium constants the influence of ligand and the nature of vinyl cores on the stability were analyzed. These results have direct implication for gold catalysis: it was demonstrated that vinyl gold intermediates bind the catalytic LAu+ species generally stronger than an alkyne (the substrate) by a factor of 106–109. This demonstrates that the formation of diaurated species from vinyl gold intermediates is thermodynamically favored in a catalytic reaction." @default.
• W2313790876 created "2016-06-24" @default.
• W2313790876 creator A5004712464 @default.
• W2313790876 creator A5033450326 @default.
• W2313790876 date "2013-03-11" @default.
• W2313790876 modified "2023-09-27" @default.
• W2313790876 title "Quantitative Evaluation of the Stability of <i>gem</i>-Diaurated Species in Reactions with Nucleophiles" @default.
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• W2313790876 doi "https://doi.org/10.1021/om400083f" @default.
• W2313790876 hasPublicationYear "2013" @default.
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