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- W2313934294 abstract "A strategy for the controlled assembly of gold nanocrystals into dispersed three-dimensional superstructures is presented. A multifunctional RAFT agent was used to prepare multiblock polystyrene (4.4-17.8 kDa) with trithiocarbonate groups as junctions between the individual blocks. Addition of these polymers to two-phase Brust-Schiffrin gold nanoparticles (4.1 nm) resulted in the formation of stable gold-nanoparticle assemblies dispersed in toluene. TEM analysis revealed that the interparticle distances in these superstructures can be tuned over an unprecedented wide range by employing multiblock polymers with an adjusted degree of polymerization and thus tailored trithiocarbonate distances. Cross-linking of the gold nanoparticles in the assemblies by multifunctional trithiocarbonates was proven by AFM showing partly preserved globular shape after deposition on a solid substrate. The reported strategy is expected to prove useful when interparticle distances in nanoparticle assemblies need to be tuned in a liquid phase or on surfaces." @default.
- W2313934294 created "2016-06-24" @default.
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- W2313934294 date "2013-11-25" @default.
- W2313934294 modified "2023-09-25" @default.
- W2313934294 title "Spherical Gold-Nanoparticle Assemblies with Tunable Interparticle Distances Mediated by Multifunctional RAFT Polymers" @default.
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- W2313934294 doi "https://doi.org/10.1021/mz400556q" @default.
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