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• W2313996475 startingPage "6337" @default.
• W2313996475 abstract "Havellockate (1) was isolated from the soft coral Sinularia granosa located on the Havellock island in the Indian Ocean. This highly compact and polyoxygenated marine diterpene bears a cis-fused hydrindane core that contains eight stereogenic centers as well as a spiro-lactone. To the best of our knowledge, no syntheses of 1 have been reported yet. Herein, we describe the synthesis of the all-carbon framework of havellockate (1) in 18 chemical operations. Our approach highlights the efficiency and utility of the hydroxy-directed Diels−Alder (HDDA) reaction to quickly access the cis-fused hydrindane core and securing the correct stereochemistry at C6 and C7. Moreover, six of the eight stereogenic centers have been installed in the correct stereochemistry." @default.
• W2313996475 created "2016-06-24" @default.
• W2313996475 creator A5016112766 @default.
• W2313996475 creator A5051316642 @default.
• W2313996475 creator A5085784374 @default.
• W2313996475 date "2010-09-03" @default.
• W2313996475 modified "2023-10-09" @default.
• W2313996475 title "Progress toward the Total Synthesis of (±)-Havellockate" @default.
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• W2313996475 doi "https://doi.org/10.1021/jo101279z" @default.
• W2313996475 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/20815361" @default.
• W2313996475 hasPublicationYear "2010" @default.
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