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• W2314095412 startingPage "1746" @default.
• W2314095412 abstract "Alkylamides (such as N,N′-dimethylformamide, N,N′-diethylformamide, and N,N′-dimethylacetamide) are aprotic solvents that are widely used in organic synthesis. These polar molecules have no electron affinity, and it is believed that irradiated liquid and solid amides stabilize excess electrons as cavity-type species analogous to hydrated and ammoniated electrons. In this study, we use isotope substitution and EPR spectroscopy to demonstrate that, in frozen amides, the suspected “cavity electron” is, in fact, a solvent-stabilized monomer anion. Our observations call into question other attributions of such features in the literature, both in low temperature solids and room temperature liquids. We also provide a general scheme describing amide radiolysis, as the related amides are used as metal ion extracting agents in nuclear separations." @default.
• W2314095412 created "2016-06-24" @default.
• W2314095412 creator A5039381027 @default.
• W2314095412 creator A5083014857 @default.
• W2314095412 date "2012-02-10" @default.
• W2314095412 modified "2023-10-14" @default.
• W2314095412 title "Electron Localization and Radiation Chemistry of Amides" @default.
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• W2314095412 doi "https://doi.org/10.1021/jp2115687" @default.
• W2314095412 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22268635" @default.
• W2314095412 hasPublicationYear "2012" @default.
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