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• W2314287736 startingPage "12911" @default.
• W2314287736 abstract "We use a classical density functional theory (DFT) to study the electric double layer formed by charged hard spheres near a planar charged surface. The DFT predictions are found to be in good agreement with recent computer simulation results. We study the capacitance of the charged hard-sphere system at a range of densities and surface charges and find that the capacitance exhibits a local minimum at low ionic densities and small electrode charge. Although this charging behavior is typical for an aqueous electrolyte solution, the local minimum gradually turns into a maximum as the density of the hard spheres increases. Charged hard spheres at high density provide a reasonable first approximation for ionic liquids. In agreement with experiment, the capacitance of this model ionic liquid double layer has a maximum at small electrode charge density." @default.
• W2314287736 created "2016-06-24" @default.
• W2314287736 creator A5028621204 @default.
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• W2314287736 date "2011-10-17" @default.
• W2314287736 modified "2023-10-03" @default.
• W2314287736 title "Density Functional Study of the Electric Double Layer Formed by a High Density Electrolyte" @default.
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• W2314287736 doi "https://doi.org/10.1021/jp2078105" @default.
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• W2314287736 hasPublicationYear "2011" @default.
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