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• W2314687130 abstract "We show that the disorder scaling of the low-temperature optical absorption linewidth of tubular molecular assemblies sharply contrasts with that known for one-dimensional aggregates. The difference can be explained by an anomalous localization of excitons, which arises from the combination of long-range intermolecular interactions and the tube's higher-dimensional geometry. As a result, the exciton density of states near the band bottom drops to zero, leading to a strong suppression of exciton localization. Our results explain the strong linear dichroism and weak exciton-exciton scattering in tubular J aggregates observed in experiments and suggest that for nanoscale wirelike applications a tubular shape is to be preferred over a truly one-dimensional chain." @default.
• W2314687130 created "2016-06-24" @default.
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• W2314687130 date "2015-04-17" @default.
• W2314687130 modified "2023-09-25" @default.
• W2314687130 title "Signature of Anomalous Exciton Localization in the Optical Response of Self-Assembled Organic Nanotubes" @default.
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• W2314687130 doi "https://doi.org/10.1103/physrevlett.114.156804" @default.
• W2314687130 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25933330" @default.
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