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- W2314831424 abstract "The temperature dependence of ionic conductivity and the static dielectric constant is examined for 0.30 m TbaTf- or LiTf-1-alcohol solutions. Above ambient temperature, the conductivity increases with temperature to a greater extent in electrolytes whose salt has a charge-protected cation. Below ambient temperature, the dielectric constant changes only slightly with temperature in electrolytes whose salt has a cation that is not charge-protected. The compensated Arrhenius formalism is used to describe the temperature-dependent conductivity in terms of the contributions from both the exponential prefactor σo and Boltzmann factor exp(−Ea/RT). This analysis explains why the conductivity decreases with increasing temperature above 65 °C for the LiTf-dodecanol electrolyte. At higher temperatures, the decrease in the exponential prefactor is greater than the increase in the Boltzmann factor." @default.
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- W2314831424 date "2012-05-04" @default.
- W2314831424 modified "2023-09-27" @default.
- W2314831424 title "Ion Transport with Charge-Protected and Non-Charge-Protected Cations in Alcohol-Based Electrolytes Using the Compensated Arrhenius Formalism. Part I: Ionic Conductivity and the Static Dielectric Constant" @default.
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- W2314831424 doi "https://doi.org/10.1021/jp209205u" @default.
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