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- W2314884098 abstract "Six members of a new family of {ONSO}-type ligands—the tetradentate-diainionic imine-thiobis(phenolate) ligands—were prepared by a two-step synthesis. Their [{ONSO}Zr(OtBu)2] complexes formed as single diastereomers with different degrees of fluxionality that depended on the substitution pattern of the two phenolate rings. The complexes were active in polymerization of l-lactide and rac-lactide. The tacticity of the poly(lactic acid) prepared from rac-lactide changed gradually from heterotactically inclined through atactic to isotactically inclined. The most flexible complex and the most rigid complex gave the highest degrees of heterotacticity and isotacticity, respectively." @default.
- W2314884098 created "2016-06-24" @default.
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- W2314884098 date "2012-01-06" @default.
- W2314884098 modified "2023-10-08" @default.
- W2314884098 title "Ring-Opening Polymerization of Lactide with Zr Complexes of {ONSO} Ligands: From Heterotactically Inclined to Isotactically Inclined Poly(lactic acid)" @default.
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- W2314884098 doi "https://doi.org/10.1021/ma2023364" @default.
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