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• W2314891207 abstract "We have investigated thermal expansion of a tetragonal ${mathrm{Mn}}_{88}{mathrm{Ni}}_{12}$ alloy by x-ray diffraction, Mn and Ni $K$-edge extended x-ray-absorption fine-structure spectroscopy, and the computational simulations based on the path-integral effective-classical-potential theory. It is found from the x-ray diffraction that the tetragonal lattice constant $c$ exhibits almost no thermal expansion like an Invar alloy, while the lattice constant $a$ shows even larger thermal expansion than usually expected from anharmonicity, implying significant anisotropy in thermal expansion. The extended x-ray-absorption fine-structure reveals that the Mn local environment is actually tetragonally distorted, while the Ni one retains its inherent cubiclike symmetry. Combined with the computational simulations, it is concluded that large thermal expansion along the $a$ axis originates from the anti-Invar effect, while negligibly small thermal expansion along the $c$ axis originates from the cooperative Invar effect. Namely, the tetragonally distorted more stable antiferromagnetic Mn state gives a significantly smaller (slightly longer) atomic radius along the $a$ ($c$) axis than the radius of the spherical paramagnetic state." @default.
• W2314891207 created "2016-06-24" @default.
• W2314891207 creator A5067233448 @default.
• W2314891207 creator A5079069492 @default.
• W2314891207 date "2013-02-13" @default.
• W2314891207 modified "2023-09-23" @default.
• W2314891207 title "Anisotropic Thermal Expansion and Cooperative Invar and Anti-Invar Effects in Mn Alloys" @default.
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• W2314891207 doi "https://doi.org/10.1103/physrevlett.110.075901" @default.
• W2314891207 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25166383" @default.
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