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- W2314930772 abstract "We have studied spin-dependent charge transfer dynamics in wirelike donor-bridge-acceptor (D-B-A) molecules comprising a phenothiazine (PTZ) donor, an oligo(2,7-fluorene) (FL(n)) bridge, and a perylene-3,4:9,10-bis(dicarboximide) (PDI) acceptor, PTZ-FL(3)-PDI (1) and PTZ-FL(4)-PDI (2), dissolved in the magnetic field-aligned nematic phase of 4-cyano-4'-n-pentylbiphenyl (5CB) at 295 K. Time-resolved EPR spectroscopy using both continuous wave and pulsed microwaves shows that the photogenerated radical pairs (RPs), PTZ(+•)-FL(3)-PDI(-•) and PTZ(+•)-FL(4)-PDI(-•), recombine much faster from the singlet RP manifold than the triplet RP manifold. When a strong resonant microwave π pulse is applied following RP photogeneration in 1 and 2, the RP lifetimes increase about 50-fold as indicated by electron spin-echo detection. This result shows that the RP lifetime can be greatly extended by rapidly switching off fast triplet RP recombination." @default.
- W2314930772 created "2016-06-24" @default.
- W2314930772 creator A5072522213 @default.
- W2314930772 creator A5076420255 @default.
- W2314930772 date "2011-02-14" @default.
- W2314930772 modified "2023-10-17" @default.
- W2314930772 title "Manipulating Photogenerated Radical Ion Pair Lifetimes in Wirelike Molecules Using Microwave Pulses: Molecular Spintronic Gates" @default.
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- W2314930772 doi "https://doi.org/10.1021/ja110789q" @default.
- W2314930772 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21319821" @default.
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