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• W2314996864 abstract "Little is known on the early stages of the methanol-to-olefin (MTO) conversion over H-SAPO-34, before the steady-state with highly active polymethylbenzenium cations as most important intermediates is reached. In this work, the formation and evolution of carbenium ions during the early stages of the MTO conversion on a H-SAPO-34 model catalyst were clarified via 1H MAS NMR and 13C MAS NMR. Several initial species (i.e., three-ring compounds, dienes, polymethylcyclopentenyl, and polymethylcyclohexenyl cations) were, for the first time, directly verified during the MTO conversion. Their detailed evolution network was established from theoretical calculations. On the basis of these results, an olefin-based catalytic cycle is proposed to be the primary reaction pathway during the early stages of the MTO reaction over H-SAPO-34. After that, an aromatic-based cycle may be involved in the MTO conversion for long times on stream." @default.
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• W2314996864 date "2014-12-09" @default.
• W2314996864 modified "2023-10-15" @default.
• W2314996864 title "Understanding the Early Stages of the Methanol-to-Olefin Conversion on H-SAPO-34" @default.
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• W2314996864 doi "https://doi.org/10.1021/cs5015749" @default.
• W2314996864 hasPublicationYear "2014" @default.
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