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- W2315483672 abstract "Abstract The synthesis and the solid state magnetic properties of (nitronyl nitroxide)‐substituted trioxytriphenylamine radical cation tetrachlorogallate, NNTOT+·GaCl4− , are reported. In the temperature region between 300 and 3 K, the magnetic behavior is characterized by the strong intramolecular ferromagnetic interaction ( J / k B =+400 K) between the radical ( NN ) and the radical cation ( TOT + ) and the weak intermolecular antiferromagnetic interaction ( J / k B =−1.9 K) between NNTOT + ions. Below 3 K, a 3D‐type long‐range magnetic ordering into a weak ferromagnet was observed ( T N =2.65 K). The magnetic entropy ( S mag =8.97 J K −1 mol −1 ) obtained by the heat capacity measurement is in good agreement with the theoretical value of R ln3=9.13 J K −1 mol −1 based on the S =1 state." @default.
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- W2315483672 date "2012-05-03" @default.
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- W2315483672 title "(Nitronyl Nitroxide)‐Substituted Trioxytriphenylamine Radical Cation Tetrachlorogallate Salt: A 2p‐Electron‐Based Weak Ferromagnet Composed of a Triplet Diradical Cation" @default.
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- W2315483672 doi "https://doi.org/10.1002/asia.201200084" @default.
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