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- W2315552008 abstract "We have extended the doorway-window representation of optical pump-probe spectroscopy with weak pulses toward N-wave-mixing spectroscopy with temporally well-separated pulses of arbitrary strength. The expressions for the signals in the strong-pulse doorway-window representation are derived in the framework of the nonperturbative theory of N-wave-mixing spectroscopy. The strong-pulse doorway-window representation is complementary to the equation-of-motion phase-matching approach. The latter fully accounts for pulse-overlap effects in signals induced by weak pulses but is computationally more expensive. The performance of the doorway-window approximation for temporally well-separated strong pulses is illustrated for an electronic two-level system with an underdamped Condon-active vibrational mode." @default.
- W2315552008 created "2016-06-24" @default.
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- W2315552008 creator A5016274435 @default.
- W2315552008 creator A5036623395 @default.
- W2315552008 date "2011-03-22" @default.
- W2315552008 modified "2023-10-16" @default.
- W2315552008 title "Optical <i>N</i>-Wave-Mixing Spectroscopy with Strong and Temporally Well-Separated Pulses: The Doorway−Window Representation" @default.
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- W2315552008 doi "https://doi.org/10.1021/jp112055h" @default.
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