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• W2315590565 abstract "The photodissociation dynamics of 2-iodotoluene following excitation at 266 nm have been investigated employing femtosecond time-resolved mass spectrometry. The photofragments are detected by multiphoton ionization using an intense laser field centered at 800 nm. A dissociation time of 380 +/- 50 fs was measured from the rising time of the co-fragments of toluene radical (C7H7) and iodine atom (I), which is attributed to the averaged time needed for the C-I bond breaking for the simultaneously excited n sigma* and pi* states by 266 nm pump light. In addition, a probe light centered at 298.23 nm corresponding to resonance wavelength of ground-state iodine atom is used to selectively ionize ground-state iodine atoms generated from the dissociation of initially populated n sigma* and pi pi* states. And a rise time of 400 50 fs is extracted from the fitting of time-dependent I+ transient, which is in agreement with the dissociation time obtained by multiphoton ionization with 800 nm, suggesting that the main dissociative products are ground-state iodine atoms." @default.
• W2315590565 created "2016-06-24" @default.
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• W2315590565 date "2016-02-27" @default.
• W2315590565 modified "2023-09-23" @default.
• W2315590565 title "Photodissociation Dynamics of 2-Iodotoluene Investigated by Femtosecond Time-Resolved Mass Spectrometry" @default.
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• W2315590565 doi "https://doi.org/10.1063/1674-0068/29/cjcp1512243" @default.
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