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- W2315927219 abstract "A series of three chiral, expanded six-membered NHC–palladium(II) complexes was prepared with successively increased sterical demand, while retaining natural d-(+)-camphor as a chiral motif. The catalysts showed different reaction profiles in the asymmetric, intramolecular α-arylation of amides. The molecular structure of two N-heterocyclic and one nitrogen acyclic carbene palladium isonitrile complex was unequivocally determined by X-ray crystallographic analysis. The results reported herein account for a correlation of catalytic activity and enantiodiscrimination in relation to the degree of chiral substitution and steric congestion at the metal center. The modular and convergent synthetic route of these air- and moisture-stable palladium isonitrile complexes underlines the usefulness of this approach." @default.
- W2315927219 created "2016-06-24" @default.
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- W2315927219 date "2012-01-30" @default.
- W2315927219 modified "2023-10-18" @default.
- W2315927219 title "Six-Membered, Chiral NHCs Derived from Camphor: Structure–Reactivity Relationship in Asymmetric Oxindole Synthesis" @default.
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- W2315927219 doi "https://doi.org/10.1021/om201166b" @default.
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