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• W2316026064 abstract "We report ${}^{11}mathrm{B}$ nuclear magnetic resonance (NMR) and zero-field muon spin relaxation (ZF-$ensuremath{mu}mathrm{SR})$ measurements of the anisotropic spin tetramer system ${mathrm{CdCu}}_{2}phantom{rule{0.16em}{0ex}}({mathrm{BO}}_{3}){phantom{rule{0.16em}{0ex}}}_{2}$, which consists of strongly interacting Cu(1) dimers and weakly coupled nonfrustrated Cu(2) spins. Long-range magnetic order is observed at ${T}_{N}=9.8$ K by a critical divergence of the nuclear spin-lattice relaxation rate $1/{T}_{1}$ and an appearance of well-defined muon-spin precessions. In addition, we find the spectroscopic signature for a magnetic anomaly at ${T}^{*}=6.5$ K, a few kelvins below ${T}_{N}$. For temperatures below ${T}^{*},1/{T}_{1}$ ceases to follow a ${T}^{4.9(1)}$ behavior. Instead, upon cooling below ${T}^{*}$, both $1/{T}_{1}$ and $1/{T}_{2}$ become temperature-independent with a subsequent small drop. The muon frequency and the relative fraction of the Cu magnetic sites show anomalies mostly for Cu(2) spins at ${T}^{*}$. This is ascribed to a Cu(2) spin reorientation. Site-specific change in magnetic structure is discussed in terms of the energy hierarchy of involved exchange interactions and an additional intertetramer interaction that controls magnetism at temperature ${T}^{*}$." @default.
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• W2316026064 date "2014-12-04" @default.
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• W2316026064 title "Anomalous spin dynamics in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mi>CdCu</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>BO</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:mo>)</mml:mo><mml:msub><mml:mrow /><mml:mn>2</mml:mn></mml:msub></mml:math>revealed by<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msup><mml:mrow /><mml:mn>11</mml:mn></mml:msup><mml:mi mathvariant=normal>B</mml:mi></mml:mrow></mml:math>NMR and …" @default.
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• W2316026064 doi "https://doi.org/10.1103/physrevb.90.214416" @default.
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