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- W2316106648 abstract "A series of novel one-dimensional (1D) lanthanide coordination polymers, [Ln(pqc)(Hpqc)(NO3)2]n (Ln = Sm (1), Eu (2), Gd (3), Tb (4), Dy (5), Ho (6), Er (7), Tm (8), Yb (9), or Lu (10); Hpqc = 2-phenyl-4-quinolinecarboxylic acid), have been synthesized via solvothermal reaction at low temperature and then characterized by single-crystal X-ray diffraction. Polymers 1–10 are isostructural and feature a 1D chain based on binuclear units in which Ln3+ polyhedra are interconnected by bridging Hpqc ligands and terminal nitrates. The infinite chains are further extended to a three-dimensional supramolecular framework through π···π stacking and hydrogen bonding interactions. This series affords an opportunity to study the lanthanide contraction effect, demonstrating that the sum of Ln–O distances proportional to this contraction follow a quadratic decay as a function of the number n of f electrons. The photoluminescence spectra show that these complexes are highly sensitized by Hpqc and exhibit characteristic Ln3+ (Sm (1), Eu (2), Tb (4), Er (7), and Yb (9)) and ligand centered (Dy (5), Ho (6), Tm (8), and Lu (10)) luminescence in both visible and near-infrared (NIR) regions. The magnetic properties of 4–7 have also been investigated." @default.
- W2316106648 created "2016-06-24" @default.
- W2316106648 creator A5022899451 @default.
- W2316106648 creator A5026733759 @default.
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- W2316106648 creator A5048511806 @default.
- W2316106648 creator A5076300428 @default.
- W2316106648 creator A5079034428 @default.
- W2316106648 creator A5083582614 @default.
- W2316106648 creator A5084329352 @default.
- W2316106648 date "2013-11-13" @default.
- W2316106648 modified "2023-09-27" @default.
- W2316106648 title "Crystal Structure, Multiplex Photoluminescence, and Magnetic Properties of a Series of Lanthanide Coordination Polymers Based on Quinoline Carboxylate Ligand" @default.
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